Peer-Review Publications

Recently, the contribution of the generalized Breit interaction to electron impact ionization was identified for the first time in a high‐Z system, namely, hydrogen‐like uranium. This study employed a measurement of the relative population of the j = 1/2 and j = 3/2 states of the L shell by projectile excitation in collision of U91+ with hydrogen and nitrogen targets. However, for a rigorous test of ion–atom collision theory, also the absolute excitation cross sections are of great importance. In the present work, we report on our efforts to extend the previous study to a determination of the absolute projectile excitation cross sections by normalization to the well‐known radiative electron capture process.

The atomic physics collaboration SPARC is a part of the APPA pillar at the future Facility for Antiproton and Ion Research. It aims at atomic‐physics research across virtually the full range of atomic matter. An emphasis of this contribution are the atomic physics experiments addressing the collision dynamics in strong electro‐magnetic fields as well as the fundamental interactions between electrons and heavy nuclei at the HESR. Here we give a short overview about the central instruments for SPARC experiments at this storage ring.

We study the trident process in laser pulses. We provide exact numerical results for all contributions, including the difficult exchange term. We show that all terms are in general important for a short pulse. For a long pulse, we identify a term that gives the dominant contribution even if the intensity is only moderately high, a0≳1, which is an experimentally important regime where the standard locally constant field (LCF) approximation cannot be used. We show that the spectrum has a richer structure at a0∼1, compared to the LCF regime a0≫1. We study the convergence to LCF as a0 increases and how this convergence depends on the momentum of the initial electron. We also identify the terms that dominate at high energy.

An ultrafast laser delivering 10.4 kW average output power based on a coherent combination of 12 step-index fiber amplifiers is presented. The system emits close-to-transform-limited 254 fs pulses at an 80 MHz repetition rate, and has a high beam quality (M2 ≤ 1.2) and a low relative intensity noise of 0.56% in the frequency range of 1 Hz to 1 MHz. Automated spatiotemporal alignment allows for hands-off operation.

We report an analysis of electron‐optical properties of a toroidal magnetic sector spectrometer and examine parameters for its implementation in a relativistic heavy‐ion storage ring, for example the High Energy Storage ring (HESR) at the future Facility for Antiproton and Ion Research (FAIR) facility. For studies of free–free pair production in heavy‐ion atom collisions, this spectrometer exhibits very high efficiencies for coincident e+–e− pair spectroscopy over a wide range of momenta of emitted lepton pairs. The high coincidence efficiency of the spectrometer is the key for stringent tests of theoretical predictions for the phase space correlation of lepton vector momenta in free–free pair production.

High-energy completeness of quantum electrodynamics (QED) can be induced by an interacting ultraviolet fixed point of the renormalization flow. We provide evidence for the existence of two of such fixed points in the subspace spanned by the gauge coupling, the electron mass and the Pauli spin-field coupling. Renormalization group trajectories emanating from these fixed points correspond to asymptotically safe theories that are free from the Landau pole problem. We analyze the resulting universality classes defined by the fixed points, determine the corresponding critical exponents, study the resulting phase diagram, and quantify the stability of our results with respect to a systematic expansion scheme. We also compute high-energy complete flows towards the long-range physics. We observe the existence of a renormalization group trajectory that interconnects one of the interacting fixed points with the physical low-energy behavior of QED as measured in experiment. Within pure QED, we estimate the crossover from perturbative QED to the asymptotically safe fixed point regime to occur somewhat above the Planck scale but far below the scale of the Landau pole.

The present status of the fully-relativistic nonperturbative calculations of the fundamental atomic processes with twisted electrons is presented. In particular, the elastic (Mott) scattering, the radiative recombination, and for the very first time, the Bremsstrahlung processes are considered. The electron-ion interaction is accounted for in a nonperturbative manner, that allows obtaining reliable results for heavy systems. We investigate the influence of the "twistedness" of the incoming electron on the angular and polarization properties of the emitted electrons and photons for the elastic and inelastic scattering, respectively. It is found that these properties exhibit a strong dependence on the opening angle of the vortex electron beam in all processes considered.

Synopsis We present non-destructive single-pass ion bunch detection and characterisation by measuring the induced image charge in a detection electrode. The presented technique allows direct determination of ion kinetic energy, absolute ion number and spatial ion bunch length. We will show the results of corresponding measurements with bunches of low-energy highly charged ions and discuss the minimum detectable number of charges.

We present charge‐state evolution studies for Pb⁵⁴⁺ ion beams passing through stripper foils at relativistic energies of 5.9 GeV/u. The purpose of this investigation is to determine the optimum target material and non‐equilibrium thickness for the efficient production of few‐electron lead ions, that is, Pb⁸⁰⁺ and Pb⁸¹⁺, at the present European Organization for Nuclear Research, CERN, accelerator facility at energies as high as 5.9 GeV/u. Based on these predictions, an Al stripper foil has been selected for a proof‐of‐principle measurement in the frame of the Gamma Factory study group. The experimental data confirms a substantial yield of non‐bare Pb ions. In addition, a charge‐state evolution study for the production of Li‐like lead ions Pb⁷⁹⁺ is presented, which will be subject of a follow‐up experiment in the near future.

We discuss the electron-optical properties of a toroidal magnetic sector spectrometer and its suitablilty for electron-positron pair spectroscopy in relativistic ion-atom collisions in the future HESR storage ring at FAIR. With the simultaneous mapping of electrons and positrons and geometric invariants in the lepton trajectorties this instrument offers a very high efficiency for studies of vector momentum correlation in free-free pair production.

We report on a comparative study of strong-field ionization of alkaline-earth-metal atoms by intense femtosecond laser pulses from near-infrared to midinfrared wavelengths. By collecting the ionization signals only produced within the central portion of the laser focus, the focus volume effect is largely reduced and the saturation intensities for different alkaline-earth-metal atoms are reliably determined, which permits us to directly test the strong-field-ionization theories. We demonstrate that the Perelomov-Popov-Terent'ev model accurately predicts the experimental ionization yields and saturation intensities in general for arbitrary values of the Keldysh parameter, while the Ammosov-Delone-Krainov simulations agree with the experiments for the tunneling-ionization regime and also for the regime when the Keldysh parameter is around 1. Our work presents benchmark data for strong-field ionization of alkaline-earth metals over a broad range of laser parameters and confirms the validity of Keldysh's picture for such atoms.

A concept of a high resolution asymmetric von Hamos X-ray spectrometer for the CRYRING@ESR electron cooler is described and its characteristics obtained by ray-tracing Monte-Carlo simulations are presented. The spectrometer will be used to study the QED e-ects in H-like medium-Z ions by measuring the energies of X-rays from radiative recombination of highly charged ions with cooling electrons, with a ppm precision of energy determination.

Luminosity is a measure of the colliding frequency between beam and target and it is a crucial parameter for the measurement of absolute values, such as reaction cross sections. In this paper, we make use of experimental data from the ESR storage ring to demonstrate that the luminosity can be precisely determined by modelling the measured Rutherford scattering distribution. The obtained results are in good agreement with an independent measurement based on the x-ray normalization method. Our new method provides an alternative way to precisely measure the luminosity in low-energy stored-beam configurations. This can be of great value in particular in dedicated low-energy storage rings where established methods are difficult or impossible to apply.

The exact knowledge of optical material parameters is crucial for laser systems design. Therefore, the work reported herein was dedicated to the determination of an important parameter that is typically not known or only known with insufficient precision: the Kerr coefficient determined by the third order non-linearity, also called the n2-parameter. The optical Kerr effect is responsible for the accumulated nonlinear phase (the B-integral) in high energy laser amplifiers, which often represents a serious limitation. Therefore, the knowledge of n2 is especially required for new types of laser materials. In this paper we report measurements carried out on the widely used optical material Ytterbium-doped Yttrium Aluminium Garnet (Yb:YAG) ceramics. Furthermore, the new Neodymium-doped Calcium Fluoride (Nd:CaF2) crystal was investigated. Specifically, three different approaches have been employed to determine experimentally the nonlinear refractive index of these materials. Thus classical Z-scan technique (at two different wavelengths), the degenerated four waves mixing and the time-resolved digital holography techniques, were compared. These different approaches have permitted the precise measurements of these parameters as well as their dispersion estimations.

A detector setup for registering ion species between the poles of a dipole magnet at CRYRING@ESR has been developed. It is based on a scintillator delivering light via a quartz light guide onto a semiconductor photomultiplier. The detector is capable of operating in a strong magnetic field. It can be swiftly retracted from the exposition area during the beam injection into the ring and repositioned back for the measurement cycle to avoid unnecessary exposition and, thus, to increase the scintillator life time.

In this work, we demonstrate a discrete dispersion scan scheme using a low number of flat windows to vary the dispersion of laser pulses in discrete steps. Monte Carlo simulations indicate that the pulse duration can be retrieved accurately with less than 10 dispersion steps, which we verify experimentally by measuring few-cycle pulses and material dispersion curves at 3 and 10 µm wavelength. This minimal measuring scheme using only five optical components without the need for linear positioners and interferometric alignment can be readily implemented in many wavelength ranges and situations.

Scattering of light on relativistic heavy ion beams is widely used for characterizing and tuning the properties of both the light and the ion beam. Its elastic component-Rayleigh scattering-is investigated in this work for photon energies close to certain electronic transitions because of its potential usage in the Gamma Factory initiative at CERN. The angle-differential cross-section, as well as the degree of polarization of the scattered light are investigated for the cases of 1s - 2p1/2 and 1s - 2p3/2 resonance transitions in H-like lead ions. In order to gauge the validity and uncertainty of frequently used approximations, we compare different methods. In particular, rigorous quantum electrodynamics calculations are compared with the resonant electric-dipole approximation evaluated within the relativistic and nonrelativistic formalisms. For better understanding of the origin of the approximation, the commonly used theoretical approach is explained here in detail. We find that in most cases, the nonrelativistic resonant electric-dipole approximation fails to describe the properties of the scattered light. At the same time, its relativistic variant agrees with the rigorous treatment within a level of 10% to 20%. These findings are essential for the design of an experimental setup exploiting the scattering process, as well as for the determination of the scattered light properties.

We present a study of laser-driven ion acceleration with micrometre and sub-micrometre thick targets, which focuses on the enhancement of the maximum proton energy and the total number of accelerated particles at the PHELIX facility. Using laser pulses with a nanosecond temporal contrast of up to and an intensity of the order of, proton energies up to 93 MeV are achieved. Additionally, the conversion efficiency at incidence angle was increased when changing the laser polarization to p, enabling similar proton energies and particle numbers as in the case of normal incidence and s-polarization, but reducing the debris on the last focusing optic.

A compact, femtosecond-pumped noncollinear optical parametric amplifier (NOPA) is presented with a passive spectral shaping technique, employed to produce a flat-top-like ultrabroadband output spectrum. The NOPA is pumped by a dedicated 2 mJ, 120 fs Yb3+- based CPA system, which generates both the second harmonic pump pulse and white light supercontinuum as the signal pulse. A chirped mirror pair pre-compensates the material GVD within the optical path of the signal pulse to produce a near-FTL pulse duration at the OPA crystal output. By optimizing both the pump/signal cross angle and the pump/signal delay, the 40 cm × 40 cm footprint, single-pass, fs-pumped, direct NOPA (non-NOPCPA) system generates a record 20 μJ, 11 fs pulses at 820 nm central wavelength with a bandwidth of 230 nm FWHM, to be used as an ultrashort optical probe pulse for relativistic laser-plasma interactions at the petawatt-class POLARIS laser system.

We present on THz generation in the two-color gas plasma scheme driven by a high-power, ultrafast fiber laser system. The applied scheme is a promising approach for scaling the THz average power but it has been limited so far by the driving lasers to repetition rates up to 1 kHz. Here, we demonstrate recent results of THz generation operating at a two orders of magnitude higher repetition rate. This results in a unprecedented THz average power of 50 mW. The development of compact, table-top THz sources with high repetition rate and high field strength is crucial for studying nonlinear responses of materials, particle acceleration or faster data acquisition in imaging and spectroscopy.

We present a flexible all-polarization-maintaining (PM) mode-locked ytterbium (Yb):fiber laser based on a nonlinear amplifying loop mirror (NALM). In addition to providing detailed design considerations, we discuss the different operation regimes accessible by this versatile laser architecture and experimentally analyze five representative mode-locking states. These five states were obtained in a 78-MHz configuration at different intracavity group delay dispersion (GDD) values ranging from anomalous (-0.035 ps2) to normal (+0.015 ps2). We put a particular focus on the characterization of the intensity noise as well as the free-running linewidth of the carrier-envelope-offset (CEO) frequency as a function of the different operation regimes. We observe that operation points far from the spontaneous emission peak of Yb (~1030 nm) and close to zero intracavity dispersion can be found, where the influence of pump noise is strongly suppressed. For such an operation point, we show that a CEO linewidth of less than 10-kHz at 1 s integration can be obtained without any active stabilization.

Theoretical g-factor calculations for the first excited 2P3/2 state of boronlike ions in the range Z=10–20 are presented and compared with the previously published values. The first-order interelectronic-interaction contribution is evaluated within the rigorous quantum electrodynamics (QED) approach in the effective screening potential. The second-order contribution is considered within the Breit approximation. The QED and nuclear recoil corrections are also taken into account.

We present a novel, to the best of our knowledge, Hartmann wave front sensor for extreme ultraviolet (EUV) spectral range with a numerical aperture (NA) of 0.15. The sensor has been calibrated using an EUV radiation source based on gas high harmonic generation. The calibration, together with simulation results, shows an accuracy beyond λ/39 root mean square (rms) at λ = 32 nm. The sensor is suitable for wave front measurement in the 10 nm to 45 nm spectral regime. This compact wave front sensor is high-vacuum compatible and designed for in situ operations, allowing wide applications for up-to-date EUV sources or high-NA EUV optics.

We present a carrier-envelope phase (CEP)-stable Yb-doped fiber laser system delivering 100 µJ few-cycle pulses at a repetition rate of 100 kHz. The CEP stability of the system when seeded by a carrier-envelope offset-locked oscillator is 360 mrad, as measured pulse-to-pulse with a stereographic above-threshold ionization (stereo-ATI) phase meter. Slow CEP fluctuations have been suppressed by implementing a feedback loop from the phase meter to the pulse picking acousto-optic modulator. To the best of our knowledge, this is the highest CEP stability achieved to date with a fiber-based, high-power few-cycle laser.

A micro-calorimeter X-ray detector of the maXs-30 type was used to record the X-ray radiation from Fe ions, being produced in the S-EBIT-I electron beam ion trap at the site of GSI. The resulting spectra demonstrate the superior energy resolving power of micro-calorimeter detectors compared with conventional semiconductor detectors. The experiment serves as another proof of principle for the application of calorimeters as dedicated high-resolution X-ray spectrometers at an ion facility. Together with the development of an improved analysis algorithm for online readout, these results present a step towards the use of maXs-type detectors as standard instrumentation at GSI/FAIR.