Peer-Review Publications

We describe a novel method to improve the temporal intensity contrast (TIC) between the main pulse and prepulses in a high-power chirped-pulse amplification (CPA) laser system. Pre- and post-pulses originating from the limited extinction ratio of the polarization gating equipment are suppressed by carefully adjusting the round-trip times of the regenerative amplifiers (RAs) with respect to the oscillator. As a result, leaking pulses from earlier or later round-trips in the RAs are hidden below the temporal shape of the main pulse. The synchronization can easily be controlled by a contrast measurement on a picosecond time scale using a third-order cross-correlator that enables a sub-mm precise adjustment of the cavity lengths. Finally, a method based on spectral interference is introduced that can be used for a fine-adjustment of the cavity lengths for the daily operation, making this new method easy to implement into existing laser systems.

Electron acceleration by laser-driven plasma waves is capableof producing ultra-relativistic, quasi-monoenergetic electron bunches with orders of magnitude higher accelerating gradients and much shorter electron pulses than state-of-the-art radio-frequency accelerators. Recent developments have shown peak energies reaching into the GeV range and improved stability and control over the energy spectrum and charge. Future applications, such as the development of laboratory X-ray sources with unprecedented peak brilliance or ultrafast time-resolved measurements critically rely on a temporal characterization of the acceleration process and the electron bunch. Here, we report the first real-time observation of the accelerated electron pulse and the accelerating plasma wave. Our time-resolved study allows a single-shot measurement of the (5.8_(−2.1))^(+1.9) fs electron bunch full-width at half-maximum ((2.5_(−0.9))^(+0.8) fs root mean square) as well as the plasma wave with a density-dependent period of 12–22 fs and reveals the evolution of the bunch, its position in the surrounding plasma wave and the wake dynamics. The results afford promise for brilliant, sub-ångström-wavelength ultrafast electron and photon sources for diffraction imaging with atomic resolution in space and time.

We report on a Yb:YAG Innoslab laser amplifier system for generation of subpicsecond high energy pump pulses for optical parametric chirped pulse amplification (OPCPA) at high repetition rates. Pulse energies of up to 20 mJ (at 12.5 kHz) and repetition rates of up to 100 kHz were attained with pulse durations of 830 fs and average power in excess of 200 W. We further investigate the possibility to use subpicosecond pulses to derive a stable continuum in a YAG crystal for OPCPA seeding.

Monitoring of beam currents in particle accelerators without affecting the beam guiding elements, interrupting the beam or influencing its profile is a major challenge in accelerator technology. A solution to this problem is the detection of the magnetic field generated by the moving charged particles. We present a non-destructive beam monitoring system for particle beams in accelerators based on the Cryogenic Current Comparator (CCC) principle. The CCC consists of a high-performance low-temperature DC superconducting quantum interference device (LTS DC-SQUID) system, a toroidal pick-up coil, and a meander-shaped superconducting niobium shield. This device allows the measurement of continuous as well as pulsed beam currents in the nA-range. The resolution and the frequency response of the detector strongly depend on the toroidal pick-up coil and its embedded ferromagnetic core. Investigations of both the temperature and frequency dependence of the relative permeability and the noise contribution of several nanocrystalline ferromagnetic core materials are crucial to optimize the CCC with respect to an improved signal-to-noise ratio and extended transfer bandwidth.

The absorption of an ultra-intense circularly-polarized laser pulse by a near-critical (0.1 n_c < n_e < a_0 n_c) plasma is studied. Previously two regimes of absorption have been suggested: a 'leading edge depletion' (LED) regime and a 'transverse ponderomotive acceleration' regime. Here we seek to describe these concepts more thoroughly, and determine if two distinct regimes actually exist. New analytic models to describe each regime are derived. These are compared with 1D and 2D particle-in-cell simulations, and good quantitative agreement is found, showing the existence of two separate regimes. The LED regime exhibits very efficient absorption of laser light, which is promising for applications.

Some features of charge-changing processes, namely, electron capture (EC) and electron loss (EL), are considered for heavy many-electron ions colliding with neutral atoms in a wide range of ion energy E = 10 keV/u – 100 GeV/u. The discussion is based on cross-section calculations performed by available computer codes, namely, CAPTURE, DEPOSIT and RICODE. The RICODE (Relativistic Ionization CODE), which provides calculation of single-electron loss cross sections in the relativistic energy regime, was recently created on the basis of the relativistic Born approximation and is described in the Appendix A. In addition, a semi-empirical formula for single-electron loss cross sections is suggested based on properties of the Born approximation and numerical calculations by the RICODE program. To cover also the low and intermediate collision energies, EL cross sections are obtained by the recently created DEPOSIT code which provides calculation of single- and multiple-electron as well as the total cross sections. Based on the results obtained by these codes, recommended capture and loss cross sections for heavy ions like xenon, uranium and lead ions colliding with neutral atoms are presented over a wide energy range.

We present the first clear identification and highly accurate measurement of the intra-shell transition 1s2p^3P_2 → 1s2s^3S_1 of He-like uranium performed via x-ray spectroscopy. The present experiment was conducted at the gas-jet target of the ESR storage ring in GSI (Darmstadt, Germany), where a Bragg spectrometer, with a bent germanium crystal, and a Ge(i) detector were mounted. Using the ESR deceleration capabilities, we performed a differential measurement between the 1s2p^3P_2→1s2s^3S_1 He-like U transition energy, at 4510 eV, and the 1s^2 2p^2P_(3/2) → 1s^2 2s^2S_(1/2) Li-like U transition energy, at 4460 eV. By a proper choice of the ion velocities, the x-ray energies from the He- and Li-like ions could be measured, in the laboratory frame, at the same photon energy. This allowed for a drastic reduction of experimental systematic uncertainties, principally due to the Doppler effect, and for a comparison with theory without the uncertainties arising from one-photon quantum electrodynamics predictions and nuclear size corrections.

Heavy few-electron ions, such as He-, Li- and Be-like ions, are ideal atomic systems to study the effects of correlation, relativity and quantum electrodynamics. Very recently, theoretical and experimental studies of these species achieved a considerable improvement in accuracy. Be-like ions are interesting because their first excited state, i.e. (1s2 2s2p)3P0, has an almost infinite lifetime (τ0) in the absence of nuclear spin (I), as it can only decay by a two-photon E1M1 transition to the (1s2 2s2)1S0 ground state. In addition, the energy difference between the 3P0 and the next higher-lying 3P1 state is expected to remain almost completely unaffected by QED effects, and should thus be dominated by the effects of correlation and relativity. Therefore, we want to determine the (1s2 2s2p) 3P0–3P1 level splitting in Be-like krypton (84Kr32+), which has I=0, by means of laser spectroscopy at the experimental storage ring at GSI. In such an experiment, the energy splitting can be obtained with very good accuracy and can be compared with recent calculations.

We present here a Monte Carlo program based on the EGS5 package for modeling the detector response of position-sensitive x-ray detectors. The program is used to estimate the polarimeter quality of two novel detector systems applied in Compton polarimetry. The validity of the underlying physical models is verified by comparing the simulation output to experimental data obtained at the experimental storage ring, ESR.

Photonic-Crystal Fibers (PCF) are among the most promising concepts to achieve large mode field areas suitable for the reduction of nonlinearities in fibers. Differential mode propagation loss is the cornerstone of effective single-mode behavior in passive and core-pumped active PCFs. In this work, we explore non-hexagonal PCF designs with increased mode discrimination in comparison to the classical hexagonal PCF designs. It is shown that a pentagonal design can increase the mode discrimination and, simultaneously, also improve the beam quality of Large-Pitch Fibers with mode field diameters well beyond 100 µm.

We observed the x-ray emission of 191.7 MeV u^(−1) Li-like uranium associated with resonant coherent excitation from 1s^(2) 2s to 1s^(2) 2p_(3/2) (4459 eV) in a thin silicon crystal target. De-excitation x-rays were observed by using large-area silicon drift detectors installed inside the target vacuum chamber together with their preamplifiers. We found that the x-ray yield under the resonance condition was clearly enhanced by a factor of three compared to that under the random incidence condition.

The linear polarization of bremsstrahlung radiation emitted in collisions of spin‐polarized and unpolarized electrons with carbon and gold targets has been measured for an incident kinetic energy of 100 keV. We present preliminary results for the degree of linear polarization for incident unpolarized electrons as a function of bremsstrahlung photon energy.

The future international accelerator Facility for Antiproton and Ion Research (FAIR) encompasses 4 scientific pillars containing at this time 14 approved technical proposals worked out by more than 2000 scientists from all over the world. They offer a wide range of new and challenging opportunities for atomic physics research in the realm of highly‐charged heavy ions and exotic nuclei. As one of the backbones of the Atomic, Plasma Physics and Applications (APPA) pillar, the Stored Particle Atomic Physics Research Collaboration (SPARC) has organized tasks and activities in various working groups for which we will present a concise survey on their current status.

When a laser pulse hits a solid surface with relativistic intensities, XUV attosecond pulses are generated in the reflected light. We present an experimental and theoretical study of the temporal properties of attosecond pulse trains in this regime. The recorded harmonic spectra show distinct fine structures which can be explained by a varying temporal pulse spacing that can be controlled by the laser contrast. The pulse spacing is directly related to the cycle-averaged motion of the reflecting surface. Thus the harmonic spectrum contains information on the relativistic plasma dynamics.

We present a plasma mirror configuration that improves the temporal pulse contrast of femtosecond terawatt laser pulses by a factor of thousand using a single antireflection coated glass target. The device provides ultra-high contrast for experiments with a maximum repetition rate of 10 Hz. A third-order cross-correlator has been used to measure the temporal pulse contrast for several different plasma mirror targets. It is shown that the ASE can be suppressed to a level of 10^(−11.) A comparison between a triggered and an untriggered plasma mirror reveals differences in the intensity distribution of the focused beam. The triggered plasma mirror produces a slightly larger focus due to the expansion of the triggered plasma mirror at -3 ps before the main pulse. We propose a cost-effective AR-coated and a blank glass target to reduce the costs of the consumable target material. High-harmonic radiation on solid surfaces has been generated with different plasma mirror targets to demonstrate the high laser contrast.

In this paper a scheme is proposed for measuring nuclear-spin-dependent parity-nonconservation effects in highly charged ions. The idea is to employ circularly polarized laser light for inducing the transition between the level (1s2s)^1S_0 and the hyperfine sublevels of (1s2s)^3S_1 in He-like ions with nonzero nuclear spin. We argue that an interference between the allowed magnetic dipole M1 and the parity-violating electric dipole E1 decay channel leads to an observable asymmetry of order 10^(-7) in the transition cross section, in the atomic range 28 ⩽ Z ⩽ 35. Experimental requirements for asymmetry measurements are discussed in the case of He-like (34)_Se^(77).

Due to electron-nucleus weak interaction, atomic bound states with different parities turn out to be mixed. We discuss a prospective method for measuring the mixing parameter between the nearly degenerate metastable states 1s_(1/2) 2s_(1/2):J=0 and 1s_(1/2) 2p_(1/2):J=0 in heliumlike uranium. Our analysis is based on the polarization properties of the photons emitted in the two-photon decays of such states.

The population of magnetic sublevels in hydrogen-like uranium ions has been investigated in relativistic ion–atom collisions by observing the subsequent X-ray emission. Using the gas target at the experimental storage ring facility we observed the angular emission of Lyman-α radiation from hydrogen-like uranium ions. The alignment parameter for three different interaction energies was measured and found to agree well with theory. In addition, the use of different gas targets allowed for the electron-impact excitation process to be observed.

We demonstrate that an ultrashort-pulse laser-driven x-ray diode can be used for time-resolved experiments on a picosecond timescale. Hence, acoustical phonons in germanium are observed after ultrashort laser-excitation and the results are compared with calculations according to a microphysical model. We also show the advantages of this kind of picosecond x-ray source compared to other sources on the basis of its properties.

We present simple and compact (1.5 m x 0.5 m footprint) post-compression of a state-of-the-art fiber chirped pulse amplification system. By using two stage nonlinear compression in noble gas filled hollow core fibers we shorten 1 mJ, 480 fs, 50 kHz pulses. The first stage is a 53 cm long, 200 µm inner diameter fiber filled with xenon with subsequent compression in a chirped mirror compressor. A 20 cm, 200 µm inner diameter fiber filled with argon further broadens the spectrum in a second stage and compression is achieved with another set of chirped mirrors. The average power is 24.5 W / 19 W after the first / second stage, respectively. Compression to 35 fs is achieved. Numerical simulations, agreeing well with experimental data, yield a peak power of 5.7 GW at a pulse energy of 380 µJ making this an interesting source for high harmonic generation at high repetition rate and average power.

We report on the design and experimental investigation of a preferential gain photonic-crystal fiber with a mode-field diameter of 47 µm. This few-mode fiber design confines the doping of Ytterbium-ions just to the center of the core and, therefore, promotes fundamental mode operation. In a chirped-pulse amplification system we extracted up to 303 W of average power from this fiber with a measured M^2 value of 1.4.

We describe the optical pump–probe laser system at the XUV free-electron laser FLASH at DESY. A growing interest in optical laser pulses combined with the free-electron laser (FEL) beam for time-resolved experiments raise high demands on the stability of operation and knowledge on the status of synchronization between the XUV and optical pulses. In this publication we describe this system, the characterization of the optical pulses, synchronization and timing schemes as well as beamlines that transport beam to experimental stations.

Experimental results in laser acceleration of protons and ions and theoretical predictions that the currently achieved energies might be raised by factors 5 - 10 in the next few years have stimulated research exploring this new technology for oncology as a compact alternative to conventional synchrotron based accelerator technology. The emphasis of this paper is on collection and focusing of the laser produced particles by using simulation data from a specific laser acceleration model. We present a scaling law for the “chromatic emittance” of the collector - here assumed as a solenoid lens - and apply it to the particle energy and angular spectra of the simulation output. For a 10 Hz laser system we find that particle collection by a solenoid magnet well satisfies requirements of intensity and beam quality as needed for depth scanning irradiation. This includes a sufficiently large safety margin for intensity, whereas a scheme without collection - by using mere aperture collimation - hardly reaches the needed intensities.

In an article “Lorentz violation in high-energy ions” by S. Devasia published in this Journal [EPJ C 69, 343 (2010)], our recent Doppler shift experiments on fast ion beams are reanalyzed. Contrary to our analysis, Devasia concludes that our results provide an “indication of Lorentz violation”. We argue that this conclusion is based on a fundamental misunderstanding of our experimental scheme and reiterate that our results are in excellent agreement with Special Relativity.

Fourth-generation X-ray light sources are being developed to deliver laser-like X-ray pulses at intensities and/or repetition rates that are beyond the reach of table-top devices. An important class of experiments at these new facilities comprises pump–probe experiments, which are designed to investigate chemical reactions and processes occurring on the molecular or even atomic level, and on the timescale of a few femtoseconds. Good progress has been made towards the generation of ultrashort X-ray pulses (for example, at FLASH or LCLS), but experiments suffer from the intrinsic timing jitter between the X-ray pulses and external laser sources3. In this Letter, we present a new approach that provides few-femtosecond temporal resolution. Our method uses coherent terahertz radiation generated at the end of the X-ray undulator by the same electron bunch that emits the X-ray pulse. It can therefore be applied at any advanced light source working with ultrashort electron bunches and undulators.