Referierte Publikationen

We report on the dynamics of ultrafast heating in cryogenic hydrogen initiated by a ≲300  fs, 92 eV free electron laser x-ray burst. The rise of the x-ray scattering amplitude from a second x-ray pulse probes the transition from dense cryogenic molecular hydrogen to a nearly uncorrelated plasmalike structure, indicating an electron-ion equilibration time of ∼0.9  ps. The rise time agrees with radiation hydrodynamics simulations based on a conductivity model for partially ionized plasma that is validated by two-temperature density-functional theory.

Abstract The generation of intense ion beams from high-intensity laser-generated plasmas has been the focus of research for the last decade. In the LIGHT collaboration the expertise of heavy ion accelerator scientists and laser and plasma physicists has been combined to investigate the prospect of merging these ion beams with conventional accelerator technology and exploring the possibilities of future applications. We report about the goals and first results of the LIGHT collaboration to generate, handle and transport laser driven ion beams. This effort constitutes an important step in research for next generation accelerator technologies.

SPARC collaboration at FAIR pursues the worldwide unique research program by utilizing storage ring and trapping facilities for highly-charged heavy ions. The main focus is laid on the exploration of the physics at strong, ultra-short electromagnetic fields including the fundamental interactions between electrons and heavy nuclei as well as on the experiments at the border between nuclear and atomic physics. Very recently SPARC worked out a realization scheme for experiments with highly-charged heavy-ions at relativistic energies in the High-Energy Storage Ring HESR and at very low-energies at the CRYRING coupled to the present ESR. Both facilities provide unprecedented physics opportunities already at the very early stage of FAIR operation. The installation of CRYRING, dedicated Low-energy Storage Ring (LSR) for FLAIR, may even enable a much earlier realisation of the physics program of FLAIR with slow anti-protons.

Spin dynamics and induced spin effects in above-threshold ionization of hydrogenlike highly charged ions in super-strong laser fields are investigated. Spin-resolved ionization rates in the tunnelling regime are calculated by employing two versions of a relativistic Coulomb-corrected strong-field approximation (SFA). An intuitive simpleman model is developed which explains the derived scaling laws for spin flip and spin asymmetry effects. The intuitive model as well as our ab initio numerical simulations support the analytical results for the spin effects obtained in the dressed SFA where the impact of the laser field on the electron spin evolution in the bound state is taken into account. In contrast, the standard SFA is shown to fail in reproducing spin effects in ionization even at a qualitative level. The anticipated spin-effects are expected to be measurable with modern laser techniques combined with an ion storage facility.

Various ternary aluminosilicate glasses with the molar compositions 20 Al2O3-60 SiO2-20 R2O (R = Li or Na), 20 Al2O3-60 SiO2-20 RO (R = Mg, Ca or Zn) and 23.1 Al2O3-69.2 SiO2-7.7 R2O3 (R = Y or La) doped with 1 [times] 1020 Sm3+ cm-3 or 1 [times] 1020 Eu3+ cm-3 (about 0.2 mol% Sm2O3 or Eu2O3) were prepared. The glasses were studied with respect to their molecular structure, and their thermo-mechanical and fluorescence properties. All glasses show relatively broad fluorescence excitation and only a weak effect of the glass composition on the emission spectra is observed. Although the glasses should be structurally very similar, huge differences are found in the coefficients of thermal expansion and the glass transition temperatures. The fluorescence lifetime increases steadily with decreasing mean atomic weight and decreasing refractive index of the glasses, which may be explained by local field effects. The only exception from this rule is the zinc aluminosilicate glass, which shows a relatively high fluorescence lifetime. The highest fluorescence lifetime is found for the lithium aluminosilicate glass. The lowest coefficients of thermal expansion are found for zinc- and magnesium aluminosilicate glasses. A low coefficient of thermal expansion is a prerequisite for a high thermal shock resistance of the material and hence favorable for high-power laser applications.

X-ray emission from hollow ions offers new diagnostic opportunities for dense, strongly coupled plasma. We present extended modeling of the x-ray emission spectrum reported by Colgan et al. [Phys. Rev. Lett. 110, 125001 (2013)] based on two collisional-radiative codes: the hybrid-structure Spectroscopic Collisional-Radiative Atomic Model (SCRAM) and the mixed-unresolved transition arrays (MUTA) ATOMIC model. We show that both accuracy and completeness in the modeled energy level structure are critical for reliable diagnostics, investigate how emission changes with different treatments of ionization potential depression, and discuss two approaches to handling the extensive structure required for hollow-ion models with many multiply excited configurations.

Electron-positron pair production in oscillating electric fields is investigated in the nonperturbative threshold regime. Accurate numerical solutions of quantum kinetic theory for corresponding observables are presented and analyzed in terms of a proposed model for an effective mass of electrons and positrons acquired within the given strong electric field. Although this effective mass cannot provide an exact description of the collective interaction of a charged particle with the strong field, physical observables are identified which carry direct and sensitive signatures of the effective mass.

Divided-pulse amplification is a promising method for the energy scaling of femtosecond laser amplifiers, where pulses are temporally split prior to amplification and coherently recombined afterwards. We present a method that uses an actively stabilized setup with separated stages for splitting and combining. The additional degrees of freedom can be employed to mitigate the limitations originating from saturation of the amplifier that cannot be compensated in passive double-pass configurations using just one common stage for pulse splitting and combining. In a first proof-of-principle experiment, actively controlled divided pulses are applied in a fiber chirped-pulse amplification system resulting in combined and compressed pulses with an energy of 1.25 mJ and a peak power of 2.9 GW.

We report, for the first time, the generation of high-order harmonics in a spectral range between 200 eV and 1 keV with an unusual spectral property: only every 4th (4i + 1, i∈ℵ) harmonic line appears, whereas the usual high-harmonic spectra consist of every odd (2i + 1) harmonic. We attribute this unique property to the quantum path interference of two extended electron trajectories that experience multiple re-scattering. In the well-established theory, electrons emitted via tunnel ionisation are accelerated by a laser field, return to the ion and recombine. The acceleration typically lasts for less than one optical cycle, and the electrons radiate in the extreme ultraviolet range at recombination. In contrast, for extended trajectories, electrons are accelerated over two or more optical cycles. Here, we demonstrate that two sets of trajectories dominate and provide substantial contributions to the generated soft X-ray radiation because they fulfil the resonance condition for X-ray parametric amplification.

The angular distribution of the Kα_1 (1s2p_3/2^1,3P_1,2→1s^21S_0) x-ray emission following the radiative electron capture into initially hydrogenlike ions with nonzero nuclear spin has been studied within the density matrix theory and the multiconfiguration Dirac-Fock method. Emphasis is placed especially upon the hyperfine interaction and how this interaction of the magnetic moment of the nucleus with those of the electrons affects the angular properties of the Kα_1 radiation. Calculations were performed for selected isotopes of heliumlike Sn48+, Xe52+, and Tl79+ ions. A quite sizable contribution of the hyperfine interaction upon the Kα_1 angular emission is found for isotopes with nuclear spin I = 1/2, while its effect is suppressed for (most) isotopes with nuclear spin I > 1/2. We therefore suggest that accurate measurements of the Kα_1 angular distribution at ion storage rings can be utilized as a tool for determining the nuclear parameters of rare stable and radioactive isotopes with I ≥ 1/2.

In this work we numerically study the evolution and interaction of one-dimensional (1-D) dark spatial solitons and semi-infinite dark stripes (SIDSs) in a local self-defocusing Kerr nonlinear medium. The experimental results in the linear regime of propagation confirm that the SIDS bending and fusion with the infinite 1-D dark beam modeled for negative nonlinearity is due to the opposite phase semi-helicities of SID beam ends. Results for several interaction scenaria show that bending ends of the semi-infinite dark stripes splice to the 1-D dark beam to form structures resembling waveguide couplers/branchers. Well pronounced modulational stability of 1-D dark spatial solitons under strong symmetric background beam modulation from decaying SIDSs is predicted.

The Compton scattering of x-ray photons, assisted by a short intense optical laser pulse, is discussed. The differential scattering cross section reveals the interesting feature that the main Klein-Nishina line is accompanied by a series of side lines forming a broad plateau where up to O(10^(3)) laser photons participate simultaneously in a single scattering event. An analytic formula for the width of the plateau is given. Due to the nonlinear mixing of x-ray and laser photons a frequency-dependent rotation of the polarization of the final-state x-ray photons relative to the scattering plane emerges. A consistent description of the scattering process with short laser pulses requires to work with x-ray pulses. An experimental investigation can be accomplished, e.g., at LCLS or the European XFEL, in the near future.

We experimentally investigate the ionization mechanism behind the formation of remarkably high charge states observed in the laser-pulse-induced fragmentation of different hydrocarbon molecules by Roither et al. [Phys. Rev. Lett. 106, 163001 (2011)], who suggested enhanced ionization occurring at multiple C-H bonds as the underlying ionization mechanism. Using multiparticle coincidence momentum imaging we measure the yield of multiply charged fragmenting ethylene and acetylene molecules at several intensities and pulse durations ranging from the few-cycle regime to 25 fs. We observe, at constant intensity, a strong increase of the proton energy with increasing laser pulse duration. It is shown that this is caused by a strong increase in the yield of highly charged parent molecular ions with pulse duration. Based on experimental evidence we explain this increase by the necessary population of precursor states in the parent ion that feature fast C-H stretch dynamics to the critical internuclear distance, where efficient ionization via enhanced ionization takes place. For increasing pulse duration these precursor ionic states are more efficiently populated, which leads in turn to a higher enhanced-ionization probability for longer pulses. Our work provides experimental evidence for the existence of a multiple-bond version of enhanced ionization in polyatomic molecules.

The Feynman tools have been re-designed with the goal to establish and implement a high-level (computer) language that is capable to deal with the physics of finite, n -qubit systems, from frequently required computations to mathematically advanced tasks in quantum information processing. In particular, emphasis has been placed to introduce a small but powerful set of keystring-driven commands in order to support both, symbolic and numerical computations. Though the current design is implemented again within the framework of Maple, it is general and flexible enough to be utilized and combined with other languages and computational environments. The present implementation facilitates a large number of computational tasks, including the definition, manipulation and parametrization of quantum states, the evaluation of quantum measures and quantum operations, the evolution of quantum noise in discrete models, quantum measurements and state estimation, and several others. The design is based on a few high-level commands, with a syntax close to the mathematical notation and its use in the literature, and which can be generalized quite readily in order to solve computational tasks at even higher degree of complexity. In this work, I present and discuss the (re-design of the) Feynman tools and make major parts of the code available for public use. Moreover, a few selected examples are shown and demonstrate possible application of this toolbox. The Feynman tools are provided as Maple library and can hence be used on all platforms on which this computer-algebra system is accessible.

We report on the development of new materials for laser-ion acceleration applicable for the advanced mechanism of radiation-pressure-acceleration. These targets are ultra-thin with thicknesses of just a few nm. For several years, diamond-like carbon foils in this thickness range can be produced. An alternative material containing more than one ion-species has the potential to further improve the acceleration mechanism. The fabrication and characterization of self-supporting polymer-based targets will be described in this paper. Furthermore, we show the significant influence on a radiation-pressure induced acceleration process by experimental data.

Multielectron coincidence spectroscopy has been used to study core 4f valence 5d, 6s double photoionization of atomic mercury. Multiconfiguration Dirac–Fock calculations were performed to calculate the energies and to estimate the single-photon intensities of the 4f^13(5d^96s^2 + 5d^106s^1) double-ionized states of atomic mercury. Reasonable agreement between the measured and simulated spectra is found if the relaxation effects of the bound-state density is taken into account in the computation of the photoionization amplitudes.

A conceptual design of a high power, ultrabroadband optical parametric chirped-pulse amplifier(OPCPA) was carried out comparing nonlinear crystals (LBO and BBO) for 810 nm centered, sub-7.0 fspulses with energies above 1 mJ. These amplifiers are only possible with a parallel development ofkilowatt-level OPCPA-pump amplifiers. It is therefore important to know good strategies to use theavailable OPCPA-pump energy efficiently. Numerical simulations, including self- and cross-phasemodulation, were used to investigate the critical parameters to achieve sufficient spectral andspatial quality. At high output powers, thermal absorption in the nonlinear crystals starts todegrade the output beam quality. Strategies to minimize thermal effects and limits to the maximumaverage power are discussed.

A three-stage heavy ion acceleration scheme for generation of high-energy quasimonoenergetic heavy ion beams is investigated using two-dimensional particle-in-cell simulation and analytical modeling. The scheme is based on the interaction of an intense linearly polarized laser pulse with a compound two-layer target (a front heavy ion layer + a second light ion layer). We identify that, under appropriate conditions, the heavy ions preaccelerated by a two-stage acceleration process in the front layer can be injected into the light ion shock wave in the second layer for a further third-stage acceleration. These injected heavy ions are not influenced by the screening effect from the light ions, and an isolated high-energy heavy ion beam with relatively low-energy spread is thus formed. Two-dimensional particle-in-cell simulations show that ∼100 MeV/u quasimonoenergetic Fe^24+ beams can be obtained by linearly polarized laser pulses at intensities of 1.1×10^21W/cm2.

We present a novel ytterbium (Yb)-doped large-pitch fiber design with significantly increased pump absorption and higher energy storage/gain per unit length, which enables high-peak-power fiber laser systems with smaller footprints. Up to now index matching between core and surrounding material in microstructured fibers was achieved by co-doping the active core region with fluorine. Here we carry out the index matching by passively doping the cladding with germanium, thus raising its index of refraction. Hence, the fluorine in the core can be omitted, which leads to an effective increase of the core doping concentration, while detrimental effects such as photo-darkening and lifetime quenching are avoided by maintaining the bulk Yb concentration. Experiments and simulations show that a gain higher than 50  dB/m and an output average power higher than 100 W with excellent beam quality are feasible even with a fiber length of only 40 cm.

Temporal evolution of plasma jets from micrometre-scale thick foils following the interaction of intense (3 × 10 20 W cm^−2 ) laser pulses is studied systematically by time resolved optical interferometry. The fluid velocity in the plasma jets is determined by comparing the data with 2D hydrodynamic simulation, which agrees with the expected hole-boring (HB) velocity due to the laser radiation pressure. The homogeneity of the plasma density across the jets has been found to be improved substantially when irradiating the laser at circular polarization compared to linear polarization. While overdense plasma jets were formed efficiently for micrometre thick targets, decreasing the target areal density and/or increasing the irradiance on the target have provided indication of transition from the ‘HB’ to the ‘light sail (LS)’ regime of RPA, characterized by the appearance of narrow-band spectral features at several MeV/nucleon in proton and carbon spectra.

We present a tabletop source of coherent soft x-ray radiation with high-photon flux. Two-cycle pulses delivered by a fiber-laser-pumped optical parametric chirped-pulse amplifier operating at 180 kHz repetition rate are upconverted via high harmonic generation in neon to photon energies beyond 200 eV. A maximum photon flux of 1.3 x 10^8  photons/s is achieved within a 1% bandwidth at 125 eV photon energy. This corresponds to a conversion efficiency of ~10^−9, which can be reached due to a gas jet simultaneously providing a high target density and phase matching. Further scaling potential toward higher photon flux as well as higher photon energies are discussed.

We report on recent experimental results concerning the generation of collimated (divergence of the order of a few mrad) ultra-relativistic positron beams using a fully optical system. The positron beams are generated exploiting a quantum-electrodynamic cascade initiated by the propagation of a laser-accelerated, ultra-relativistic electron beam through high- Z solid targets. As long as the target thickness is comparable to or smaller than the radiation length of the material, the divergence of the escaping positron beam is of the order of the inverse of its Lorentz factor. For thicker solid targets the divergence is seen to gradually increase, due to the increased number of fundamental steps in the cascade, but it is still kept of the order of few tens of mrad, depending on the spectral components in the beam. This high degree of collimation will be fundamental for further injection into plasma-wakefield afterburners.

The (elastic) Rayleigh scattering of hard x rays by hydrogenlike ions has been investigated within the framework of second-order perturbation theory and Dirac's relativistic equation. The focus of this study was, in particular, on two questions: (i) How is the polarization of scattered photons affected if the incident light is itself (linearly) polarized, and (ii) how do the nondipole contributions to the electron-photon interaction and the relativistic contraction of the wave functions influence such a polarization transfer? Detailed calculations were performed for Ne9+, Xe53+, and U91+ targets and for photon energies up to ten times the 1s ionization threshold of the ions. From the comparison of these fully relativistic computations with the (nonrelativistic) dipole approximation we conclude that relativistic and higher-multipole effects often lead to a significant or even complete depolarization for heavy targets and at high photon energies.

We present the first direct experimental test of the complex ion structure in liquid carbon at pressures around 100 GPa, using spectrally resolved x-ray scattering from shock-compressed graphite samples. Our results confirm the structure predicted by ab initio quantum simulations and demonstrate the importance of chemical bonds at extreme conditions similar to those found in the interiors of giant planets. The evidence presented here thus provides a firmer ground for modeling the evolution and current structure of carbon-bearing icy giants like Neptune, Uranus, and a number of extrasolar planets.

The energy scaling of ultrashort-pulse systems employing simultaneously the techniques of chirped-pulse amplification and passively combined divided-pulse amplification is analyzed both experimentally and numerically. The maximum achievable efficiency is investigated and fundamental limitations originating from gain saturation, self-phase modulation and depolarization are discussed. A solution to these limitations could be an active stabilization scheme, which would allow for the operation of every single fiber amplifier at higher pulse energies.