Referierte Publikationen

We are currently devising the open-endcap Penning trap experiment (high-intensity laser ion-trap experiment) as a tool for ion confinement, manipulation and detection to be used at high-energy and/or high-intensity laser facilities. This instrument will allow studies of laser–ion interactions with well-defined ion targets, and to detect the reaction products non-destructively. The ion target may be controlled concerning the constituent species, the density, shape and position with respect to the laser focus. For commissioning experiments, we optimize the focusing parameters to achieve a high number of ionized particles per shot. The detection electronics is designed to measure all charge states of all nuclei up to xenon. We plan first experiments with argon and xenon irradiated by a titanium:sapphire chirped-pulse-amplification laser system with 10 mJ pulse energy and a pulse duration of 30 fs.

The hyperfine transitions in lithium-like and hydrogen-like bismuth were remeasured by direct laser spectroscopy at the experimental storage ring. For this we have now employed a voltage divider which enabled us to monitor the electron cooler voltage in situ . This will improve the experimental accuracy by about one order of magnitude with respect to our previous measurement using the same technique.

In this work, we report on an experiment that investigated the elastic scattering of linearly polarized 175 keV photons on a gold target. A combined measurement of the angular distribution and the linear polarization of the scattered photons was performed using standard germanium detectors and a double-sided Si(Li) strip polarimeter. Since the data analysis is still in progress, we will show results in forthcoming papers and present here how the polarimeter was used to identify a lack of shielding during the experiment.

High energy storage ring (HESR) as a part of the future accelerator facility FAIR (Facility for Antiproton and Ion Research) will serve for a variety of internal target experiments with high-energy stored heavy ions (SPARC collaboration). Bare uranium is planned to be used as a primary beam. Since a storage time in some cases may be significant—up to half an hour—it is important to examine the high-order effects in the long-term beam dynamics. A new ion optics specifically for the heavy ion mode of the HESR is developed and is discussed in this paper. The subjects of an optics design, tune working point and a dynamic aperture are addressed. For that purpose nonlinear beam dynamics simulations are carried out. Also a flexibility of the HESR ion optical lattice is verified with regard to various experimental setups. Specifically, due to charge exchange reactions in the internal target, secondary beams, such as hydrogen-like and helium-like uranium ions, will be produced. Thus the possibility of separation of these secondary ions and the primary U⁹²⁺ beam is presented with different internal target locations.

Laser cooling is a powerful technique to reduce the longitudinal momentum spread of stored relativistic ion beams. Based on successful experiments at the experimental storage ring at GSI in Darmstadt, of which we show some important results in this paper, we present our plans for laser cooling of relativistic ion beams in the future heavy-ion synchrotron SIS100 at the Facility for Antiproton and Ion Research in Darmstadt.

High order harmonics generated at relativistic intensities have long been recognized as a route to the most powerful extreme ultraviolet pulses. Reliably generating isolated attosecond pulses requires gating to only a single dominant optical cycle, but techniques developed for lower power lasers have not been readily transferable. We present a novel method to temporally gate attosecond pulse trains by combining noncollinear and polarization gating. This scheme uses a split beam configuration which allows pulse gating to be implemented at the high beam fluence typical of multi-TW to PW class laser systems. Scalings for the gate width demonstrate that isolated attosecond pulses are possible even for modest pulse durations achievable for existing and planned future ultrashort high-power laser systems. Experimental results demonstrating the spectral effects of temporal gating on harmonic spectra generated by a relativistic laser plasma interaction are shown.

We present a theoretical analysis of the fine-structure transitions for helium-like heavy ions with non-zero nuclear spin. The angular distribution of these transitions is studied for its sensitivity with regard to the nuclear magnetic dipole moment. Detailed calculations, performed for the helium-like Sn48+, Xe52+ and Tl79+ ions with nuclear spin I=1/2, indicate that the emission pattern of the fine-structure resolved photons is significantly affected by the nuclear magnetic dipole moment and that this effect can be addressed experimentally at present storage ring facilities.

Astrophysical x-ray bursts are thought to be a result of thermonuclear explosions on the atmosphere of an accreting neutron star. Between these bursts, energy is thought to be generated by the hot CNO cycles. The ¹⁵O(α,γ)¹⁹Ne reaction is one reaction that allows breakout from these CNO cycles and into the rp-process to fuel outbursts. The reaction is expected to be dominated by a single 3/2⁺ resonance at 4.033 MeV in ¹⁹Ne, however, limited information is available on this key state. This work reports on a pioneering study of the ²⁰Ne(p,d)¹⁹Ne reaction, performed in inverse kinematics at the experimental storage ring (ESR) as a means of accessing the astrophysically important 4.033 MeV state in ¹⁹Ne. The unique, background free, high luminosity conditions of the storage ring were utilized for this, the first transfer reaction performed at the ESR. The results of this pioneering test experiment are presented along with suggestions for future measurements at storage ring facilities.

The energy loss of light ions in dense plasmas is investigated with special focus on low to medium projectile energies, i.e., at velocities where the maximum of the stopping power occurs. In this region, exceptionally large theoretical uncertainties remain and no conclusive experimental data are available. We perform simulations of beam-plasma configurations well suited for an experimental test of ion energy loss in highly ionized, laser-generated carbon plasmas. The plasma parameters are extracted from two-dimensional hydrodynamic simulations, and a Monte Carlo calculation of the charge-state distribution of the projectile ion beam determines the dynamics of the ion charge state over the whole plasma profile. We show that the discrepancies in the energy loss predicted by different theoretical models are as high as 20-30%, making these theories well distinguishable in suitable experiments.

We present novel high photon flux XUV and soft x-ray sources based on high harmonic generation (HHG). The sources employ femtosecond fiber lasers, which can be operated at very high (MHz) repetition rate and average power (>100 W). HHG with such lasers results in ∼1013 photons s−1 within a single harmonic line at ∼40 nm (∼30 eV) wavelength, a photon flux comparable to what is typically available at synchrotron beam lines. In addition, resonant enhancement of HHG can result in narrow-band harmonics with high spectral purity—well suited for precision spectroscopy. These novel light sources will enable seminal studies on electronic transitions in highly-charged ions. For example, at the experimental storage ring 2s1/2– 2p1/2 transitions in Li-like ions can be excited up to Z=47 (∼100 eV transition energy), which provides unique sensitivity to quantum electro-dynamical effects and nuclear corrections. We estimate fluorescence count rates of the order of tens per second, which would enable studies on short-lived isotopes as well. In combination with the Doppler up-shift available in head-on excitation at future heavy-ion storage rings, such as the high energy storage ring, even multi-keV transitions can potentially be excited. Pump–probe experiments with femtosecond resolution could also be feasible and access the lifetime of short-lived excited states, thus providing novel benchmarks for atomic structure theory.

The introduction of cryogenically cooled, few micrometer-sized nozzle geometries and an essential modification of the experimental storage ring (ESR) target station allowed for a reliable operation using low- Z gases at target area densities in the range of 10¹³—10¹⁴ cm−². Therefore, a remarkably versatile target source was established, enabling operation over the whole range of desired target gases (from H₂ to Xe) and area densities (~10¹⁰ to ~10¹⁴ cm−²). Moreover, the considerably smaller orifice diameter of the new target source enables a much more compact inlet chamber while, at the same time, maintaining the demanding vacuum requirements of a storage ring. A completely new inlet chamber design is presented here, which, besides the improvements regarding the achievable area densities, will feature a variable beam width down to 1 mm at the ion beam interaction region. This is of paramount importance with respect to the realization of high precision experiments, e.g. by reducing the inaccuracy of the observation angle causing the relativistic Doppler broadening. While being intended for the deployment at the future high energy storage ring within the SPARC collaboration, the new inlet chamber can also replace the current one at the ESR or serve as an internal target for CRYRING.

An automated test platform aiming at accurate and efficient cavity characterizations has recently been set up at GSI, Darmstadt. In this proceeding the composition of such a system, on both hardware and software sides, is described in detail. The amount of necessary human work is significantly reduced to the minimum, while the measurement precision is improved considerably.

We report on the experimental realization of a compact, fiber-based, ultrashort-pulse laser system in the 2 μm wavelength region delivering 24 fs pulse duration with 24 MW pulse peak power and 24.6 W average power. This performance level has been enabled by the favorable quadratic wavelength-dependence of the self-focusing limit, which has been experimentally verified to be at approximately 24 MW for circular polarization in a solid-core fused-silica fiber operated at a wavelength around 2 μm. The anomalous dispersion in this wavelength region allows for a simultaneous nonlinear spectral broadening and temporal pulse compression. This makes an additional compression stage redundant and facilitates a very simple and power-scalable approach. Simulations that include both the nonlinear pulse evolution and the transverse optical Kerr effect support the experimental results.

The FOCAL experiment involves a highly accurate twin crystal spectrometer, designed for the measurement of the ground state Lamb shift of stored highly charged ions, like hydrogen-like Au 78+, via spectroscopy in the hard-x-ray regime with an accuracy down to the few-eV level where higher-order QED contributions become accessible. For this level of accuracy all geometrical parameters including the position of the x-ray source are of crucial importance. In this conference proceeding we present our efforts to characterize the internal gas target at the experiment storage ring at GSI Darmstadt where in 2012 the FOCAL experiment was conducted.

A brief review about topical developments in the exploitation of the resonant electron–ion collision process of dielectronic recombination (DR) as a sensitive spectroscopic tool is given. The focus will be on DR storage-ring experiments of few-electron highly charged ions. Among others, the questions addressed in these studies cover diverse topics from the areas of strong-field quantum electrodynamics, of lifetime studies using DR resonances, and of nuclear physics. Examples from the storage rings CRYRING in Stockholm, TSR in Heidelberg, and ESR in Darmstadt are given. In addition, an overview is provided about the ongoing developments and future perspectives of DR collision spectroscopy at the upcoming Facility for Antiproton and Ion Research in Darmstadt, Germany.

Metallic magnetic calorimeters are energy dispersive particle detectors that are operated at temperatures below 100 mK. Applied to x-ray spectroscopy they combine the high energy resolution of crystal spectrometers with the large energy bandwidth of semiconductor detectors. After the absorption of a photon its energy is converted into heat. A paramagnetic alloy converts the temperature change into a change of magnetization that is read out by a sensitive superconducting quantum interference device magnetometer. With such a metallic magnetic calorimeter we performed two successful measurements at the internal gas target of the experimental storage ring at GSI. In the first beamtime lithium-like Au-ions were targeted on a N2 and a Xe gas target, respectively. In the second beamtime we observed a projectile beam of bare Xe ions interacting with a Xe gas target. In both experiments we achieved an energy resolution below 60 eV from 0 keV to 60 keV . We were able to detect K-lines of Xe ions of different charge states, including the Lyman series up to Ly-η and could resolve the Ly-β-doublet in H-like Xe.

The coherent combination of ultra short laser pulses is a promising approach for scaling the average and peak power of ultrafast lasers. Fiber lasers and amplifiers are especially suited for this technique due to their simple singe-pass setups that can be easily parallelized. Here we propose the combination of the well-known approach of spatially separated amplification with the technique of divided-pulse amplification, i.e. an additionally performed temporally separated amplification. With the help of this multidimensional pulse stacking, laser systems come into reach capable of emitting 10’s of joules of energy at multi-kW average powers that simultaneously employ a manageable number of fibers.

The photoionization of H+2 molecular ions is investigated for Bessel beams of twisted light. In particular, the angle-differential photoionization cross sections are evaluated for a macroscopic target of randomly distributed but initially aligned ions by using the nonrelativistic first-order perturbation theory. Detailed calculations of these cross sections and angular distributions are performed for different setups of the electron detectors and for selected opening angles of the Bessel beams and are compared with those for incident plane-wave radiation. It is shown that the modification in the angular distributions of the photoelectrons can be understood quite easily from the variations in the intensity pattern of the Bessel beams, relative to the size of the H+2 molecular ions.

High-harmonic generation (HHG) has been established as an indispensable tool in optical spectroscopy. This effect arises for instance upon illumination of a noble gas with sub-picosecond laser pulses at focussed intensities significantly greater than 1012W/cm2. HHG provides a coherent light source in the extreme ultraviolet (XUV) spectral region, which is of importance in inner shell photo ionization of many atoms and molecules. Additionally, it intrinsically features light fields with unique temporal properties. Even in its simplest realization, XUV bursts of sub-femtosecond pulse lengths are released. More sophisticated schemes open the path to attosecond physics by offering single pulses of less than 100 attoseconds duration. Resonant optical antennas are important tools for coupling and enhancing electromagnetic fields on scales below their free-space wavelength. In a special application, placing field-enhancing plasmonic nano antennas at the interaction site of an HHG experiment has been claimed to boost local laser field strengths, from insufficient initial intensities to sufficient values. This was achieved with the use of arrays of bow-tie-shaped antennas of ∼ 100nm in length. However, the feasibility of this concept depends on the vulnerability of these nano-antennas to the still intense driving laser light.We show, by looking at a set of exemplary metallic structures, that the threshold fluence Fth of laser-induced damage (LID) is a greatly limiting factor for the proposed and tested schemes along these lines.We present our findings in the context of work done by other groups, giving an assessment of the feasibility and effectiveness of the proposed scheme.

We report linear polarization measurements of x rays emitted due to dielectronic recombination into highly charged krypton ions. The ions in the He-like through O-like charge states were populated in an electron-beam ion trap with the electron-beam energy adjusted to recombination resonances in order to produce Ka x rays. The x rays were detected with a newly developed Compton polarimeter using a beryllium scattering target and 12 silicon x-ray detector diodes sampling the azimuthal distribution of the scattered x rays. The extracted degrees of linear polarization of several dielectronic recombination transitions agree with results of relativistic distorted-wave calculations. We also demonstrate a high sensitivity of the polarization to the Breit interaction, which is remarkable for a medium-Z element like krypton. The experimental results can be used for polarization diagnostics of hot astrophysical and laboratory fusion plasmas.

One-loop quantum electrodynamic (QED) corrections are studied for two basic atomic processes, radiative recombination of an electron with a bare nucleus and radiative decay of a hydrogenlike ion. The perturbations of the bound-state wave function and the binding energy due to the electron self-energy and the vacuum polarization are computed in the Feynman and Coulomb gauges. QED corrections induced by these perturbations are calculated for the differential cross section and the polarization of the emitted radiation in the radiative recombination of an electron and a bare uranium nuclei, as well as the corresponding corrections to the ratio of the E1 (electric dipole) and M2 (magnetic quadrupole) transition amplitudes in the 2p3/2→1s radiative decay of hydrogenlike uranium. The results obtained indicate the expected magnitude of the QED effects in these processes on a subpercent level.

During the last decades femtosecond lasers have proven their vast benefit in both scientific and technological tasks. Nevertheless, one laser feature bearing the tremendous potential for high-field applications, delivering extremely high peak and average powers simultaneously, is still not accessible. This is the performance regime several upcoming applications such as laser particle acceleration require, and therefore, challenge laser technology to the fullest. On the one hand, some state-of-the-art canonical bulk amplifier systems provide pulse peak powers in the range of multi-terawatt to petawatt. On the other hand, concepts for advanced solid-state-lasers, specifically thin disk, slab or fiber systems have shown their capability of emitting high average powers in the kilowatt range with a high wall-plug-efficiency while maintaining an excellent spatial and temporal quality of the output beam. In this article, a brief introduction to a concept for a compact laser system capable of simultaneously providing high peak and average powers all along with a high wall-plug efficiency will be given. The concept relies on the stacking of a pulse train emitted from a high-repetitive femtosecond laser system in a passive enhancement cavity, also referred to as temporal coherent combining. In this manner, the repetition rate is decreased in favor of a pulse energy enhancement by the same factor while the average power is almost preserved. The key challenge of this concept is a fast, purely reflective switching element that allows for the dumping of the enhanced pulse out of the cavity. Addressing this challenge could, for the first time, allow for the highly efficient extraction of joule-class pulses at megawatt average power levels and thus lead to a whole new area of applications for ultra-fast laser systems.

The process of recombination of a quasifree electron into a bound state of an initially bare nucleus with the simultaneous creation of a bound-electron–free-positron pair is investigated. This process is called negative-continuum-assisted dielectronic recombination (NCDR). In a typical experimental setup, the initial electron is not free but bound in a light atomic target. In the present work, we study the effects of the atomic target on the single- and double-differential cross sections of positron production in the NCDR process. Calculations are performed within the relativistic framework based on QED theory, accounting for the electron-electron interaction to first order in perturbation theory. We demonstrate how the momentum distribution of the target electrons removes the nonphysical singularity of the differential cross section which occurs for the initially free and monochromatic electrons.

Birefringence is one of the fascinating properties of the vacuum of quantum electrodynamics (QED) in strong electromagnetic fields. The scattering of linearly polarized incident probe photons into a perpendicularly polarized mode provides a distinct signature of the optical activity of the quantum vacuum and thus offers an excellent opportunity for a precision test of nonlinear QED. Precision tests require accurate predictions and thus a theoretical framework that is capable of taking the detailed experimental geometry into account. We derive analytical solutions for vacuum birefringence which include the spatio-temporal field structure of a strong optical pump laser field and an x-ray probe. We show that the angular distribution of the scattered photons depends strongly on the interaction geometry and find that scattering of the perpendicularly polarized scattered photons out of the cone of the incident probe x-ray beam is the key to making the phenomenon experimentally accessible with the current generation of FEL/high-field laser facilities.

FAIR with its intense beams of ions and antiprotons provides outstanding and worldwide unique experimental conditions for extreme matter research in atomic and plasma physics and for application oriented research in biophysics, medical physics and materials science. The associated research programs comprise interaction of matter with highest electromagnetic fields, properties of plasmas and of solid matter under extreme pressure, density, and temperature conditions, simulation of galactic cosmic radiation, research in nanoscience and charged particle radiotherapy. A broad variety of APPA-dedicated facilities including experimental stations, storage rings, and traps, equipped with most sophisticated instrumentation will allow the APPA community to tackle new challenges. The worldwide most intense source of slow antiprotons will expand the scope of APPA related research to the exciting field of antimatter.